Masses of transuranium nuclides measured with the PI-ICR technique at TRIGA-Trap


Chenmarev S., Blaum K., Block M., Cakirli R., Düllmann C. E., Gutiérrez M., ...Daha Fazla

European Physical Journal A, cilt.60, sa.10, 2024 (SCI-Expanded) identifier identifier

  • Yayın Türü: Makale / Tam Makale
  • Cilt numarası: 60 Sayı: 10
  • Basım Tarihi: 2024
  • Doi Numarası: 10.1140/epja/s10050-024-01414-3
  • Dergi Adı: European Physical Journal A
  • Derginin Tarandığı İndeksler: Science Citation Index Expanded (SCI-EXPANDED), Scopus, Academic Search Premier, Chemical Abstracts Core, INSPEC, zbMATH
  • İstanbul Üniversitesi Adresli: Evet

Özet

We have revisited the region of the actinides in the vicinity of the neutron number N=152 and conducted high-precision mass measurements using the newly implemented Phase-Imaging Ion-Cyclotron-Resonance (PI-ICR) technique. The masses of 244Pu and 249Cf were found to deviate by 5.4 and 2.9 combined sigmas, respectively, from our previous results published in 2014. This indicates the presence of systematic errors in the earlier measurements. Consequently, we decided to remeasure all the nuclides from our 2014 study, along with 248Cm, to ensure accuracy and reliability. With our greatly improved apparatus, we have measured the masses of 244Pu, 241Am, 243Am, 248Cm, and 249Cf, using 208Pb and 238U as mass references. The masses of these reference ions were recently determined with ultra-high precision at Pentatrap. Our results were implemented in the latest Atomic Mass Evaluation (AME), showing good consistency. The region related to the masses measured in this study, especially for isotopes near the N=152 deformed shell gap, is discussed in terms of two-neutron separation energies, first excited 2+ energy levels and their differentials, as well as δVpn values, the average proton-neutron interaction of the most loosely bound two nucleons.